First you have to clean the chair with an enzyme cleaner that will remove the odor completely, so it won't attract him back there. There are several, and I know people here have recommended different ones in the past that they have found to work well. I know Medusa and a couple others have an excellent list of things to help deter the inappropriate pee kitties. I know you posted that this kitty also has pooped outside of the box and that he was taken to the vet. I believe that the vet said it was a behavioral issue and recommended clomicalm. I know that you stated you were cautious of medicating him for the issues he is having, but several on here and others that I know of personally have had WONDERFUL results from using different medications to treat this problem. You may need to rethink that decision. I know that if you do a search, you'll probably find several threads that deal with this issue. If you wait a little while, you may get some other suggestions in this thread also. I hope you find something that works for you and the kitty.
ETA: I believe it is Urine Gone that I have used and that some others have recommended on here before. Although there are other cleaners that different ones prefer.
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